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11.
The presence of organic ligands (L) whose conditional stability constants (KML) are strong enough to allow them to form complexes with copper has been reported in oceanic waters. However, there is no general agreement on the distributional characteristics of such strong ligands in the water column. We present that these inconsistencies are derived from not only different analytical methods employed for their detection but also different oceanographic conditions. In particular, the nature and quantities of detectable natural ligands are affected by what kind of form the ligands are presentin situ in different marine environments, that is, chemical speciation of natural ligands (ligand speciation), which depends strongly on the variations in concentrations of coexisting trace metals. Using published data from observations in the laboratory and the field, we provide limits to the ranges of conditional stability constants of organic ligands for copper, zinc and cadmium that are detectable by the extensively used direct metal-titration method. For example, our model indicates that organic ligands for copper with log KCuL(Cu)>12.4 in surface water and with log KCuL(Cu)>9.9 in deep water might not have been detected because stronger ligands had formed complexes with ambient metalsin situ at a station in the North Pacific. The estimation suggests that there is a basinscale difference in speciation of natural organic ligands and, moreover, that this difference influences metal speciation. It is postulated that comparisons of the occurrence and levels of organic ligands might not be possible among spatially and temporally different observations without reconciliation of the effects of speciation of the ligands, even if an identical method is used in every case. 相似文献
12.
Time series of the vertical distribution of resuspended matter and bottom current were collected concurrently during summer at a few anchored stations in the Seto Inland Sea. The vertical distribution of resuspended matter was measured every hour for about one tidal cycle and the three components of current fluctuation were obtained at each sampling station. Current data at each sampling station show that the bottom is hydraulically smooth.Assuming that the averaged vertical distribution of resuspended matter for one tidal cycle shows a steady state distribution, the settling velocityWs of resuspended matter is estimated to be in the range of 1.2×10–2 to 5.7×10–2 cm sec–1 from analysis of the averaged distributions.The relation between the erosion rate and the bottom shear stress for this study area is investigated and is compared with that for other areas. The results show that the erosion of sediment in the Seto Inland Sea during summer occurs even due to the low bottom shear stress which is considered as almost smooth hydraulically. 相似文献
13.
Yutaka W. Watanabe Yoshiyuki Takahashi Takashi Kitao Koh Harada 《Journal of Oceanography》1996,52(3):301-312
Concentrations of total carbonate, alkalinity and dissolved oxygen were obtained near the 1973 GEOSECS stations in the North Pacific subpolar region north of 40°N along 175°E between 1993 and 1994. A difference of excess CO2 content between the GEOSECS and our expeditions was estimated. The maximum difference in water column inventory of excess CO2 has increased by about 280 gC m–2 above 2000 m depth which apparently means an uptake of excess CO2 taken from air to sea during the last two decades. An averaged value of the annual flux of excess CO2 at 75–1000 m depth was 8.63±2.01 gC m–2yr–1 in the North Pacific subpolar region. By introducing the annual flux of excess CO2 into a two-box model for the North Pacific subpolar region, a penetration factor of excess CO2 from air to sea was obtained to be 1.08×10–2 gC m–3ppm–1 in the North Pacific subpolar region. Based on this factor, the surface concentration of excess CO2 in the North Pacific subpolar region was estimated to be 68 mole I–1, suggesting that the North Pacific subpolar region absorbed atmospheric excess CO2 more than the saturated concentration of excess CO2. Total amount of excess CO2 taken from the North Pacific subpolar region by 1993 was estimated to be 36.2×1015 gC, which was equal to about one tenth of that released by human activities after the preindustrial era. 相似文献
14.
Effect of emersion and immersion on the porewater nutrient dynamics of an intertidal sandflat in Tokyo Bay 总被引:2,自引:0,他引:2
Tomohiro Kuwae Eiji Kibe Yoshiyuki Nakamura 《Estuarine, Coastal and Shelf Science》2003,57(5-6):929-940
Porewater nutrient dynamics during emersion and immersion were investigated during different seasons in a eutrophic intertidal sandflat of Tokyo Bay, Japan, to elucidate the role of emersion and immersion in solute transport and microbial processes. The water content in the surface sediment did not change significantly following emersion, suggesting that advective solute transport caused by water table fluctuation was negligible. The rate of change in nitrate concentration in the top 10 mm of sediments ranged from −6.6 to 4.8 μmol N l−1 bulk sed. h−1 during the whole period of emersion. Steep nutrient concentration gradients in the surface sediment generated diffusive flux of nutrients directed downwards into deeper sediments, which greatly contributed to the observed rates of change in porewater nutrient concentration for several cases. Microbial nitrate reduction within the subsurface sediment appeared to be strongly supported by the downward diffusive flux of nitrate from the surface sediment. The stimulation of estimated nitrate production rate in the subsurface layer in proportion to the emersion time indicates that oxygenation due to emersion caused changes in the sediment redox environment and affected the nitrification and/or nitrate reduction rates. The nitrate and soluble reactive phosphorus pools in the top 10 mm of sediment decreased markedly during immersion (up to 68% for nitrate and up to 44% for soluble reactive phosphorus), however, this result could not be solely explained by molecular diffusion. 相似文献
15.
Gymnodinium mikimotoi, a senior synonym ofGymnodinium nagasakiense often causes red tides in coastal waters of the western part of Japan. The photosynthetic pigment composition of two strains ofG. mikimotoi were analyzed by HPLC. They contain chlorophyllc
3 which has not been reported from dinoflagellates. They also contain fucoxanthin, 19'-hexanoyloxyfucoxanthin and 19'-butanoyloxyfucoxanthin as major carotenoides, which are anomalous in dinoflagellates. The pigment composition ofG. mikimotoi is compared with that ofGyrodinium aureolum which occur in European waters and is thought as a conspecific species withG. mikimotoi by several authors. 相似文献
16.
Iodine in sea water of the Pacific was determined with special interest in the relation between iodide and iodate in the surface water of the ocean. The result was discussed with reference to the mechanism of iodide formation proposed byTsunogai andSase. The concentration of iodide varies widely from the lower value than the detection limit to 0.21g at./l, while the concentration of total iodine is nearly constant and the mean value is 0.41g at./l. The vertical profile of iodide often shows the maximum in the surface layer. In the surface layer, the concentration of iodide is higher in warm water (0,10g at./l on the average) than that in cold water of lower temperature than 20° C (0.03g at/l). The highest concentration of iodide among the warm waters is found in the surface water of the equatorial area (0.13g at./l) where the biological productivity is also high. Iodide is generally more enriched in the water having higher biological activity even in the cold water. These results are considered to be compatible with the mechanism of iodide formation proposed. 相似文献
17.
Takashi Ichiye 《Journal of Oceanography》1977,33(4):169-182
A circular storm moves with a constant speedc along a geostrophic flow similar to a western boundary current in the upper layer of a two-layer ocean with the motionless lower layer. The linear inertia terms are retained. Effects of the current becomes more conspicuous for smallerc and insignificant forc above 10 m s–1. The inertia effects are manifested in cellular patterns of the interface perturbations with cell lengths of(c–vf
–1 in a wake of the storm with a radius of an order of 100 km, wherev is the current velocity. On the left hand edge where the flow has a strong shear, the interface displacements have large amplitudes which increase with a distance along the path in a wake of the storm. These disturbances propagate to the left of the edge within an angle of cot–1 (c
2/gH0–1), whereg is the reduced gravity andH
0 is the depth of the interface at the edge of the current. Comparison with the observations during Typhoon Trix in 1971 south of Japan suggests that fluctuations of the daily mean sea level with several days' periods observed along the southern coast of Japan may be due to the stationary oscillations of the Kuroshio caused by the inertia undulations along its left edge or due to the propagating perturbations to the left. 相似文献
18.
19.
A preliminary study of carbon system in the East China Sea 总被引:1,自引:0,他引:1
Shizuo Tsunogai Shuichi Watanabe Junya Nakamura Tsuneo Ono Tetsuro Sato 《Journal of Oceanography》1997,53(1):9-17
In the central part of the East China Sea, the activity of CO2 in the surface water and total carbonate, pH and alkalinity in the water column were determined in winter and autumn of 1993.
The activity of CO2 in the continental shelf water was about 50 ppm lower than that of surface air. This decrease corresponds to the absorption
of about 40 gC/m2/yr of atmospheric CO2 in the coastal zone or 1 GtC/yr in the global continental shelf, if this rate is applicable to entire coastal seas. The normalized
total carbonate contents were higher in the water near the coast and near the bottom. This increase toward the bottom may
be due to the organic matter deposited on the bottom. This conclusion is supported by the distribution of pH. The normalized
alkalinity distribution also showed higher values in the near-coast water, but in the surface water, indicating the supply
of bicarbonate from river water. The residence time of the East China Sea water, including the Yellow Sea water, has been
calculated to be about 0.8 yr from the excess alkalinity and the alkalinity input. Using this residence time and the excess
carbonate, we can estimate that the amount of dissolved carbonate transported from the coastal zone to the oceanic basin is
about 70 gC/m2/yr or 2 GtC/yr/area-of-global-continental-shelf. This also means that the rivers transport carbon to the oceans at a rate
of 30 gC/m2/yr of the coastal sea or 0.8 GtC/yr/ area-of-global shelf, the carbon consisting of dissolved inorganic carbonate and terrestrial
organic carbon decomposed on the continental shelf. 相似文献
20.
Masayuki Takahashi Isao Koike Takashi Ishimaru Toshiro Saino Ken Furuya Yoshihiko Fujita Akihiko Hattori Shun-ei Ichimura 《Journal of Oceanography》1980,36(4):209-216
Water plumes, 20 km long or less, identified by low temperature, high salinity and high nutrient concentrations, were observed on the eastern side of Izu Islands where the Kuroshio Current or its branch flowed eastward. The T-S diagrams and the vertical profiles of oceanographic variables indicated that the water plumes resulted from the upwelling of subsurface water. A newly formed plume, characterized by a sharp temperature front and high nutrient concentrations, contained less chlorophyll than did old plumes. It is suggested that the upwelling plumes are maintained for a period long enough to allow luxuriant growth of phytoplankton. 相似文献